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Notable differences between oxidized diruthenium complexes bridged by four isomeric diethynyl benzodithiophene ligands

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成果类型:
期刊论文
作者:
Ou, Ya-Ping;Zhang, Jing;Zhang, Fuxing;Kuang, Daizhi;Hartl, Frantisek*;...
通讯作者:
Liu, Sheng Hua;Hartl, Frantisek
作者机构:
[Ou, Ya-Ping; Zhang, Jing; Liu, Sheng Hua; Rao, Li] Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China.
[Ou, Ya-Ping; Zhang, Fuxing; Kuang, Daizhi] Hengyang Normal Univ, Coll Chem & Mat Sci, Hengyang 421008, Hunan, Peoples R China.
[Zhang, Fuxing; Kuang, Daizhi] Hengyang Normal Univ, Hunan Prov Coll, Key Lab Funct Organometall Mat, Hengyang 421008, Hunan, Peoples R China.
[Hartl, Frantisek] Univ Reading, Dept Chem, Reading RG6 6AD, Berks, England.
通讯机构:
[Liu, Sheng Hua] C
[Hartl, Frantisek] U
Cent China Normal Univ, Coll Chem, Minist Educ, Key Lab Pesticide & Chem Biol, Wuhan 430079, Peoples R China.
Univ Reading, Dept Chem, Reading RG6 6AD, Berks, England.
语种:
英文
期刊:
Dalton Transactions
ISSN:
1477-9226
年:
2016
卷:
45
期:
15
页码:
6503-6516
基金类别:
The authors acknowledge financial support from the National Natural Science Foundation of China (21272088, 21472059, 21402057), the Opening Subjects of Hunan Province Key Laboratory of Functional Organometallic Materials (No. GN15K05), the Scientific Research Foundation of Hengyang Normal University (No. 14B23), Scientific Research Project of Education Department of Hunan Province (No. 14C0168). F.H. thanks the University of Reading for the support of the Reading Spectroelectrochemistry laboratory (Project D14-015).
机构署名:
本校为其他机构
院系归属:
化学与材料科学学院
摘要:
Four new diruthenium complexes [{(η5-C5Me5)Ru(dppe)}2(μ-CΞC-L-CΞC)] featuring different bridging isomeric diethynyl benzodithiophenes viz. L = benzo[1,2-b;4,5-b′]dithiophene (complex 1), benzo[2,1-b;4,5-b′]dithiophene (complex 2), benzo[1,2-b;3,4-b′]dithiophene (complex 3) and benzo[1,2-b;4,3-b′]dithiophene (complex 4), were synthesized and characterized by molecular spectroscopic and crystallographic methods. The subtle changes in the molecular structure introduced by the diethynyl benzodithiophene isomers have a notable impact on the ...

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