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Biogeochemical influences on net methylmercury formation proxies along a peatland chronosequence

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成果类型:
期刊论文
作者:
Wang, Baolin;Zhong, Shunqing;Bishop, Kevin;Nilsson, Mats B.;Hu, Haiyan;...
通讯作者:
Shunqing Zhong
作者机构:
[Eklof, Karin; Bertilsson, Stefan; Bishop, Kevin; Akerblom, Staffan; Hu, Haiyan; Zhong, Shunqing; Wang, Baolin] Swedish Univ Agr Sci, Dept Aquat Sci & Assessment, SE-75007 Uppsala, Sweden.
[Zhong, Shunqing] Hengyang Normal Univ, Coll Geog & Tourism, Hengyang 421002, Peoples R China.
[Skyllberg, Ulf; Nilsson, Mats B.] Swedish Univ Agr Sci, Dept Forest Ecol & Management, SE-90183 Umea, Sweden.
[Hu, Haiyan] Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550081, Peoples R China.
[Bravo, Andrea G.] Inst Ciencies Mar ICM CSIC, Dept Marine Biol & Oceanog, Pg Maritim Barceloneta 37-49, E-08003 Barcelona, Catalunya, Spain.
通讯机构:
[Shunqing Zhong] C
College of Geography and Tourism, Hengyang Normal University, 421002 Hengyang, China<&wdkj&>Department of Aquatic Sciences and Assessment, Swedish University of Agricultural Sciences, SE-75007 Uppsala, Sweden
语种:
英文
关键词:
Mercury;Methylmercury;Chronosequence;Peatland;Porewater;Hg solubility;Chemical speciation
期刊:
Geochimica et Cosmochimica Acta
ISSN:
0016-7037
年:
2021
卷:
308
页码:
188-203
基金类别:
We would like to thank Tao Jiang, Liem Nguyen, Yu Song and Wei Zhu for their assistance in the laboratory, and Lucas Perreal, Camille Guyenot, Thibaut Imbert, Edward van Westrene, Marloes Arens, Mélissa Garsany, Laura Manteau, Jeanne Latour, Charles Sanseverino, Quan Zhou and Itziar Aguinaga Gil for the help with the sampling. This work was supported by the China Scholarship Council (CSC; NO. 201408520034, NO. 201508430285), the Sino-Swedish Mercury Management Research Framework (SMaReF: VR2013-6978), the National Natural Science Foundation of China (No. 41573078, 41303098 and 42077297) and the Swedish Research Council Formas (2016-00896).
机构署名:
本校为其他机构
院系归属:
地理与旅游学院
摘要:
A geographically constrained chronosequence of peatlands divided into three age classes (young, intermediate and old) was used to explore the role of biogeochemical influences, including electron donors and acceptors as well as chemical speciation of inorganic mercury (Hg(II)), on net formation of methylmercury (MeHg) as approximated by the fraction of MeHg to total mercury (THg) in the peat soil. We hypothesized that removing vascular plants would reduce availability of electron donors and thus net MeHg formation. However, we found no effect of the vascular plant removal. The sum of the poten...

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