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Atomically-dispersed manganese anchored on B,N co-doped carbon for the sensitive electrochemical detection of levodopa

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成果类型:
期刊论文
作者:
Wang, Fan;Li, Junhua;Chen, Xiangxiong;Feng, Hao;Liao, Huiyang;...
通讯作者:
Li, JH;Qian, D;Waterhouse, GIN
作者机构:
[Feng, Hao; Li, Junhua; Wang, Fan; Liao, Huiyang] Hengyang Normal Univ, Coll Chem & Mat Sci, Hengyang 421008, Peoples R China.
[Liu, Jinlong; Qian, Dong; Chen, Xiangxiong] Cent South Univ, Coll Chem & Chem Engn, Changsha 410083, Peoples R China.
[Waterhouse, Geoffrey I. N.; Waterhouse, GIN] Univ Auckland, Sch Chem Sci, Auckland 1142, New Zealand.
通讯机构:
[Li, JH ] H
[Qian, D ] C
[Waterhouse, GIN ] U
Hengyang Normal Univ, Coll Chem & Mat Sci, Hengyang 421008, Peoples R China.
Cent South Univ, Coll Chem & Chem Engn, Changsha 410083, Peoples R China.
语种:
英文
关键词:
Electrochemical sensing;Mn single-atom catalyst;Bamboo-derived carbon;Heteroatom doping;Levodopa detection
期刊:
Chemical Engineering Journal
ISSN:
1385-8947
年:
2024
卷:
481
页码:
148607
基金类别:
Acknowledgments This work was financially supported by the National Natural Science Foundation of China (No. 21505035, 51874359, 21171174), Scientific Research Foundation of Hunan Provincial Education Department (No. 21A0438), and Postgraduate Scientific Research Innovation Project of Hunan Province (No. CX20231266). Also, we are grateful to the High Performance Computing Centre of Central South University for assistance with the computations. GINW acknowledges funding support from the Royal Society Te Apārangi
机构署名:
本校为第一且通讯机构
院系归属:
化学与材料科学学院
摘要:
Metal single-atom catalysts offer the dual advantages of high electrochemical activity and near 100 % metal atom utilization, leading to their potential use in low-cost electrochemical sensor development. Herein, a novel electrocatalyst comprising atomically-dispersed Mn on B,N co-doped bamboo-derived carbon (MnSAs-BN-BC) was synthesized via a facile pyrolysis procedure. A high dispersion of Mn single atoms in MnSAs-BN-BC was confirmed by aberration-corrected transmission electron microscopy and elemental mapping. The Mn loading in the MnSAs-BN-BC determined by inductively coupled plasma mass ...

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