Metal-organic frameworks are recognized as active electrode materials for rechargeable batteries due to their structural diversity, abundant electrochemical active sites and large ion diffusion channels. Herein, nickel-terephthalic acid metal-organic frameworks (Ni-PTA MOFs) with different crystal and morphology structures are synthesized via a facile solvothermal method by simply adjusting the nature of solvent. Due to the fewest guest molecules and porous structure, the Ni-PTA resulting from the combinations of DMF and EtOH exhibits the comparatively higher chemical/thermal stability and sho...