Sugar additive with a halogen group enabling a highly reversible and dendrite-free Zn anode

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期刊论文

作者：

Xu, Weihao;Ma, Xipo;Lyu, Pengbo;Gao, Zhenren;Yan, Chunshuang*;...

通讯作者：

Yan, Chunshuang;Lv, CD

作者机构：

[Ma, Xipo; Lv, CD; Yan, Chunshuang; Lv, Chade; Yan, CS; Xu, Weihao] Harbin Inst Technol, Sch Chem & Chem Engn, State Key Lab Space Power Sources, Harbin 150001, Peoples R China.

[Ma, Xipo; Lv, CD; Yan, Chunshuang; Lv, Chade; Yan, CS; Xu, Weihao] Harbin Inst Technol, Sch Chem & Chem Engn, MIIT Key Lab Crit Mat Technol New Energy Convers, Harbin 150001, Peoples R China.

[Lyu, Pengbo] Xiangtan Univ, Sch Mat Sci & Engn, Hunan Prov Key Lab Thin Film Mat & Devices, Xiangtan 411105, Peoples R China.

[Gao, Zhenren] Hengyang Normal Univ, Coll Phys & Elect Engn, Hunan Prov Key Lab Micronano Energy Mat & Applica, Hengyang 421002, Peoples R China.

通讯机构：

[Lv, CD ; Yan, CS] H

Harbin Inst Technol, Sch Chem & Chem Engn, State Key Lab Space Power Sources, Harbin 150001, Peoples R China.

Harbin Inst Technol, Sch Chem & Chem Engn, MIIT Key Lab Crit Mat Technol New Energy Convers, Harbin 150001, Peoples R China.

语种：

英文

期刊：

REACTION CHEMISTRY & ENGINEERING

ISSN：

2058-9883

年：

2025

卷：

期：

页码：

214-223

DOI：

10.1039/d4re00366g

基金类别：

Natural Science Foundation of Hunan Province [52101246]; National Natural Science Foundation of China [YQ2022B006]; Natural Science Foundation of Heilongjiang Province, China [2023JJ40621]; Hunan Provincial Natural Science Foundation of China

机构署名：

本校为其他机构

院系归属：

物理与电子工程学院

摘要：

Aqueous zinc-ion batteries (AZBs) suffer from poor reversibility and limited lifespan due to parasitic side reactions and dendrite growth induced by active water. Although additives are widely used to address these issues by reducing the water content within the Zn-ion solvation sheaths, the strong interaction between the additives and Zn 2+ causes poor de-solvation kinetics. Here, we propose a strategy that introduces an electron-withdrawing halogen group to reduce the polarity of the sugar additive. Theoretical simulations and experimental re...

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Sugar additive with a halogen group enabling a highly reversible and dendrite-free Zn anode

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