Experimental and theoretical magneto-structural studies on the dicarboxylato-bridged nature of the dicopper(II)-based metal–organic frameworks

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成果类型：

期刊论文

作者：

Chen, Man-Sheng;Hua, Wei-Jie;Song, You;Wang, Peng;Sun, Wei-Yin*;...

通讯作者：

Sun, Wei-Yin

作者机构：

[Wang, Peng; Sun, Wei-Yin; Song, You; Chen, Man-Sheng] Nanjing Univ, Nanjing Natl Lab Microstruct, Sch Chem & Chem Engn, Coordinat Chem Inst,State Key Lab Coordinat Chem, Nanjing 210093, Jiangsu, Peoples R China.

[Chen, Man-Sheng] Hengyang Normal Univ, Dept Chem & Mat Sci, Hengyang 421008, Peoples R China.

[Hua, Wei-Jie; Zeng, Gui-Xiang; Li, Shu-Hua; Zhang, Chen-Yang] Nanjing Univ, Sch Chem & Chem Engn, Inst Theoret & Computat Chem, MOE,Key Lab Mesoscop Chem, Nanjing 210093, Jiangsu, Peoples R China.

通讯机构：

[Sun, Wei-Yin] N

Nanjing Univ, Nanjing Natl Lab Microstruct, Sch Chem & Chem Engn, Coordinat Chem Inst,State Key Lab Coordinat Chem, Nanjing 210093, Jiangsu, Peoples R China.

语种：

英文

关键词：

Copper(II) complex;Density functional theory calculation;Hydrothermal reaction;Magnetic property

期刊：

Inorganica Chimica Acta

ISSN：

0020-1693

年：

2012

卷：

387

页码：

137-144

DOI：

10.1016/j.ica.2012.01.006

基金类别：

National Natural Science Foundation of ChinaNational Natural Science Foundation of China (NSFC) [91122001, 21021062]; National Basic Research Program of ChinaNational Basic Research Program of China [2010CB923303, 2007CB925103]

机构署名：

本校为其他机构

院系归属：

化学与材料科学学院

摘要：

Two unprecedented metal-organic frameworks (MOFs) based on binuclear copper(II) second building units (SBUs), [Cu(INAIP)(dib)]·3.5H 2O (1) and [Cu(INAIP)(4,4′-bpy)]·3H 2O (2), [H 2INAIP = 5-(isonicotinamido)isophthalic acid, dib = 1,4-di(1-imidazolyl)benzene and 4,4′-bpy = 4,4′-bipyridine] have been synthesized by mixed H 2INAIP and rigid N-donor ligands with Cu(II) salt under hydrothermal conditions. Single crystal X-ray diffraction analysis revealed that the binuclear Cu(II) SBUs have similar coordination environments in complexes 1 and ...

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Experimental and theoretical magneto-structural studies on the dicarboxylato-bridged nature of the dicopper(II)-based metal–organic frameworks

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