Direct Synthesis of Phosphoryltriacetates from White Phosphorus via Visible Light Catalysis

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成果类型：

期刊论文

作者：

Chen, Yu;Liu, Wei;Huangfu, Xinlei;Wei, Junnian;Yu, Jiangxi;...

通讯作者：

Zhang, WX;Yu, JX

作者机构：

[Zhang, Wen-Xiong; Liu, Wei; Wei, Junnian; Chen, Yu; Huangfu, Xinlei] Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Minist Educ,Beijing Natl Lab Mol Sci BNLMS, Beijing 100871, Peoples R China.

[Zhang, Wen-Xiong; Liu, Wei; Wei, Junnian; Chen, Yu; Huangfu, Xinlei] Peking Univ, Coll Chem & Mol Engn, Key Lab Bioorgan Chem & Mol Engn, Minist Educ, Beijing 100871, Peoples R China.

[Yu, Jiangxi; Yu, JX] Hengyang Normal Univ, Coll Hunan Prov, Hunan Prov Key Lab Funct Met Organ Cpds, Key Lab Organometall New Mat, Hengyang 421008, Peoples R China.

通讯机构：

[Zhang, WX ] P

[Yu, JX ] H

Peking Univ, Coll Chem & Mol Engn, State Key Lab Rare Earth Mat Chem & Applicat, Minist Educ,Beijing Natl Lab Mol Sci BNLMS, Beijing 100871, Peoples R China.

Peking Univ, Coll Chem & Mol Engn, Key Lab Bioorgan Chem & Mol Engn, Minist Educ, Beijing 100871, Peoples R China.

Hengyang Normal Univ, Coll Hunan Prov, Hunan Prov Key Lab Funct Met Organ Cpds, Key Lab Organometall New Mat, Hengyang 421008, Peoples R China.

语种：

英文

关键词：

P4 activation;organophosphorus compounds;photocatalysis;white phosphorus;α-bromo esters

期刊：

CHEMISTRY-A EUROPEAN JOURNAL

ISSN：

0947-6539

年：

2024

卷：

期：

页码：

e202302289-

DOI：

10.1002/chem.202302289

基金类别：

Natural Science Foundation of China; National Key R&D Program of China [2021YFF0701600]; [22131001]; [21890721]

机构署名：

本校为通讯机构

摘要：

Direct Synthesis of Phosphoryltriacetates from White Phosphorus via Visible Light Catalysis: The reaction of P4 with α‐bromo esters using fac‐Ir(ppy)3 as the photocatalyst and blue LEDs (456 nm) as the light source was developed for the first time to afford a series of phosphoryltriacetates. This approach features mild reaction conditions and simple operational process without chlorination. Abstract Organophosphorus compounds (OPCs) are widely used in many fields. However, traditional synthetic routes in the industry usually involve multist...

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Direct Synthesis of Phosphoryltriacetates from White Phosphorus via Visible Light Catalysis

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