Ferroelectric Polarization and Single-Atom Catalyst Synergistically Promoting CO2 Photoreduction of CuBiP2Se6 - 成果

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Ferroelectric Polarization and Single-Atom Catalyst Synergistically Promoting CO₂ Photoreduction of CuBiP₂Se₆

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作者信息关键词期刊信息基础信息归属信息摘要

成果类型：

期刊论文

作者：

Jiang, Xingxing;Tan, Jieyao;Liu, Dongyu;Feng, Yexin;Chen, Ke-Qiu;...

通讯作者：

Vasenko, AS;Vasenko, Andrey S.;Chulkov, EV

作者机构：

[Tan, Jieyao; Jiang, Xingxing] Hengyang Normal Univ, Coll Phys & Elect Engn, Hengyang 421002, Peoples R China.

[Vasenko, AS; Liu, Dongyu; Vasenko, Andrey S.; Jiang, Xingxing] HSE Univ, Moscow 101000, Russia.

[Vasenko, Andrey S.; Chulkov, Evgueni V.; Vasenko, AS] Donostia Int Phys Ctr DIPC, Donostia San Sebastian 20018, Euskadi, Spain.

[Chulkov, Evgueni V.] Ctr Mixto CSIC UPV EHU, Ctr Fis Mat CFM MPC, San Sebastian 20018, Spain.

[Kazakova, Elena A.] Sechenov First Moscow State Med Univ, Dept Biochem, Moscow 119991, Russia.

通讯机构：

[Vasenko, AS ] H

[Vasenko, AS; Chulkov, EV ] D

HSE Univ, Moscow 101000, Russia.

Donostia Int Phys Ctr DIPC, Donostia San Sebastian 20018, Euskadi, Spain.

Ctr Mixto CSIC UPV EHU, Ctr Fis Mat CFM MPC, San Sebastian 20018, Spain.

语种：

英文

期刊：

Journal of Physical Chemistry Letters

ISSN：

1948-7185

年：

2024

卷：

期：

页码：

3611-3618

DOI：

10.1021/acs.jpclett.4c00687

基金类别：

Scientific Research Foundation of Hunan Provincial Education Department [23B0679]; Scientific Research Fund of Hunan Provincial Education Department [2023QD32]; Science Initiation Fund of Hengyang Normal University; Basic Research Program of HSE University

机构署名：

本校为第一机构

院系归属：

物理与电子工程学院

摘要：

Further improving the activity and selectivity of photocatalytic CO(2) reduction remains a challenge. Herein, we propose a new strategy for synergistically promoting photocatalytic CO(2) reduction by combining two-dimensional (2D) ferroelectric polarization and single-atom catalysis. Our calculations showed that the ferroelectric polarization of CuBiP(2)Se(6) provides the internal driving force for the separation and migration of photogenerated carriers, which provides a prerequisite for enhancing the photocatalytic efficiency. In addition, the introduction of single Ag atoms can act as an ele...

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Ferroelectric Polarization and Single-Atom Catalyst Synergistically Promoting CO₂ Photoreduction of CuBiP₂Se₆

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