Joule-Heated Interfacial Catalysis for Advanced Electrified Esterification with High Conversion and Energy Efficiency

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成果类型：

期刊论文

作者：

Zhang, Jifang;Zhang, Xinyuan;Shen, Yue;Fu, Bo;Wu, Yijin;...

通讯作者：

Yin, HJ;Zhao, HJ

作者机构：

[Zhang, Jifang; Shen, Yue; Yin, Huajie; Zhang, Xinyuan; Zhang, Haimin; Wang, Guozhong; Wu, Yijin; Kang, Jian] Chinese Acad Sci, CAS Ctr Excellence Nanosci, Anhui Key Lab Nanomat & Nanotechnol, Ctr Environm & Energy Nanomat,Key Lab Mat Phys,Ins, Hefei 230031, Anhui, Peoples R China.

[Zhang, Jifang; Shen, Yue; Yin, Huajie; Zhang, Haimin; Wang, Guozhong] Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China.

[Zhao, Huijun; Zhao, HJ; Fu, Bo; Kang, Jian] Griffith Univ, Ctr Catalysis & Clean Energy, Sch Environm & Sci, Gold Coast Campus, Southport, Qld 4222, Australia.

[Wu, Yijin] Hengyang Normal Univ, Coll Chem & Mat Sci, Hengyang 421001, Hunan, Peoples R China.

[Chen, Shan] Anhui Univ, Inst Phys Sci, Hefei 230039, Anhui, Peoples R China.

通讯机构：

[Zhao, HJ ] G

[Yin, HJ ] C

Chinese Acad Sci, CAS Ctr Excellence Nanosci, Anhui Key Lab Nanomat & Nanotechnol, Ctr Environm & Energy Nanomat,Key Lab Mat Phys,Ins, Hefei 230031, Anhui, Peoples R China.

Univ Sci & Technol China, Hefei 230026, Anhui, Peoples R China.

Griffith Univ, Ctr Catalysis & Clean Energy, Sch Environm & Sci, Gold Coast Campus, Southport, Qld 4222, Australia.

语种：

英文

关键词：

covalent organic framework;electrothermal reaction;esterification reaction;interfacial catalysis;Joule heating

期刊：

Advanced Materials

ISSN：

0935-9648

年：

2025

卷：

期：

页码：

e2413949

DOI：

10.1002/adma.202413949

基金类别：

National Natural Science Foundation of China; Collaborative Innovation Program of Hefei Science Center, CAS [2022HSC-CIP016]; [52301271]

机构署名：

本校为其他机构

院系归属：

化学与材料科学学院

摘要：

Esterification reactions are crucial in industries such as chemicals, fragrances, and pharmaceuticals but often face limitations due to high reversibility and low reactivity, leading to restricted yields. In this work, an electrified esterification pathway utilizing a Joule-heated interfacial catalysis (JIC) system is proposed, where a hydrophilic, sulfonic acid-functionalized covalent organic framework grown on carbon felt (COF─SO(3)H@CF) acts as the interfacial catalyst, and the carbon felt serves as the electric heat source. This approach a...

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Joule-Heated Interfacial Catalysis for Advanced Electrified Esterification with High Conversion and Energy Efficiency

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