Cationic defect-enriched hydroxides as anodic catalysts for efficient seawater electrolysis

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成果类型：

期刊论文

作者：

Wu, Yi-jin;Zheng, Jian-zhong;Zhou, Xiao;Tu, Teng-xiu;Liu, Yangyang;...

通讯作者：

Shenlong Zhao

作者机构：

[Wu, Yi-jin; Tu, Teng-xiu; Zhou, Xiao; Tan, Liang] Hengyang Normal Univ, Coll Chem & Mat Sci, Hunan Engn Res Ctr Monitoring & Treatment Heavy Me, Key Lab Funct Met Organ Cpds Hunan Prov, Hengyang 421001, Peoples R China.

[Zhao, Shenlong; Liu, Yangyang] Univ Sydney, Sch Chem & Biomol Engn, Sydney, NSW 2006, Australia.

[Zhou, Xiao] Hengyang Normal Univ, Nanyue Coll, Hengyang 421001, Peoples R China.

[Zheng, Jian-zhong] Nanjing Tech Univ, Sch Environm Sci & Engn, Nanjing 211816, Peoples R China.

[Zhang, Peng-fang] Liaocheng Univ, Sch Chem & Chem Engn, Shandong Prov Key Lab Chem Energy Storage & Novel, Liaocheng 252000, Peoples R China.

通讯机构：

[Shenlong Zhao] S

School of Chemical and Biomolecular Engineering, The University of Sydney, Sydney, NSW 2006, Australia

语种：

英文

期刊：

无机化学前沿

ISSN：

2052-1553

年：

2023

卷：

期：

页码：

2444-2456

DOI：

10.1039/d3qi00026e

基金类别：

Yi-jin Wu thanks the Scientific Research Fund of the Hunan Provincial Education Department (21B0645), the Foundation of Hunan Engineering Research Center for Monitoring and Treatment of Heavy Metals Pollution in the Upper Reaches of Xiangjiang River (2022HSKFJJ032), and the Academic College Student Innovation and Entrepreneurship Training Program (NY202123, S202210546010) for the financial support. S. Z. thanks the Australian Research Council Discovery Early Career Researcher Award (DE220100676) and the Discovery Project (DP220101511) for the financial support.

机构署名：

本校为第一机构

院系归属：

化学与材料科学学院

南岳学院

摘要：

Seawater electrocatalysis driven by renewable energy resources has long been considered as a promising approach for producing clean hydrogen. However, anodic electrode materials suffer from severe issues such as large overpotential and electrochemical corrosion during seawater electrolysis due to the existence of abundant chloride ions. Herein, we report a cationic defect engineering approach to tailoring the structure of NiFe layered double hydroxide (NiFe LDH) for the oxygen evolution reaction (OER) in an alkaline seawater-like solution. Impr...

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Cationic defect-enriched hydroxides as anodic catalysts for efficient seawater electrolysis

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