Novel hierarchical sea urchin-like Prussian blue@palladium core–shell heterostructures supported on nitrogen-doped reduced graphene oxide: Facile synthesis and excellent guanine sensing performance

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成果类型：

期刊论文

作者：

Li, Junhua;Jiang, Jianbo;Zhao, Dan;Xu, Zhifeng;Liu, Mengqin;...

通讯作者：

Qian, Dong

作者机构：

[Liu, Xing; Liu, Mengqin; Xu, Zhifeng; Li, Junhua] Hengyang Normal Univ, Coll Chem & Mat Sci, Hunan Prov Univ Key Lab Funct Organometall Mat, Key Lab Funct Met Organ Cpds Hunan Prov, Hengyang 421008, Peoples R China.

[Li, Junhua; Zhao, Dan; Qian, Dong] Cent S Univ, Coll Chem & Chem Engn, Hunan Prov Key Lab Efficient & Clean Utilizat Man, Changsha 410083, Hunan, Peoples R China.

[Jiang, Jianbo] Jishou Univ, Coll Chem & Chem Engn, Jishou 416000, Peoples R China.

[Tong, Haixia] Changsha Univ Sci & Technol, Inst Chem & Biol Engn, Changsha 410114, Hunan, Peoples R China.

通讯机构：

[Qian, Dong] C

Cent S Univ, Coll Chem & Chem Engn, Hunan Prov Key Lab Efficient & Clean Utilizat Man, Changsha 410083, Hunan, Peoples R China.

语种：

英文

关键词：

Prussian blue;Palladium;Morphology-controlled synthesis;Electrochemical detection;Guanine

期刊：

Electrochimica Acta

ISSN：

0013-4686

年：

2020

卷：

330

页码：

135196

DOI：

10.1016/j.electacta.2019.135196

基金类别：

National Natural Science Foundation of ChinaNational Natural Science Foundation of China [21505035, 51874359, 21171174, 21472038, 21603065]; Provincial Natural Science Foundation of HunanNatural Science Foundation of Hunan Province [2016JJ3028, 2017JJ2007]; Scientific Research Projects of Education Department of Hunan Province [18A336]; Hunan Provincial Science and Technology Plan Project [2016TP1007]

机构署名：

本校为第一机构

院系归属：

化学与材料科学学院

摘要：

Aiming at substantially improving the electrochemical sensing performance for guanine, we bring out a novel high-efficiency electrocatalyst composed of hierarchical sea urchin-like Prussian blue@palladium core-shell heterostructures supported on nitrogen-doped reduced graphene oxide (PB-U@Pd/N-RGO). The said PB-U@Pd/N-RGO was synthesized by a new and facile wet-chemistry method without using any surfactant and template. More impressively, we demonstrate a new strategy for morphology-controlled synthesis of Prussian blue via simply tuning the ratio of N,N'-dimethyl formamide and H2O in the mixe...

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Novel hierarchical sea urchin-like Prussian blue@palladium core–shell heterostructures supported on nitrogen-doped reduced graphene oxide: Facile synthesis and excellent guanine sensing performance

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