A self-regulated interface enabled by trivalent gadolinium ions toward highly reversible zinc metal anodes

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成果类型：

期刊论文

作者：

Zhang, Huaijun;Yang, Hengyu;Liang, Yongle;Niu, Fengjun;Xu, Guobao;...

通讯作者：

Yang, Liwen

作者机构：

[Liang, Yongle; Zhang, Huaijun; Yang, Hengyu; Niu, Fengjun] School of Physics and Optoelectronics, Xiangtan University, Xiangtan 411105, China

[Xu, Guobao] School of Materials Science and Engineering, Xiangtan University, Xiangtan 411105, China

[Wei, Xiaolin] College of Physics and Electronics Engineering, Hengyang Normal University, Hengyang 421002, China

[Yang, Liwen] School of Physics and Optoelectronics, Xiangtan University, Xiangtan 411105, China. Electronic address: ylwxtu@xtu.edu.cn

通讯机构：

[Yang, Liwen] S

School of Physics and Optoelectronics, Xiangtan University, Xiangtan 411105, China. Electronic address:

语种：

英文

关键词：

Aqueous zinc ion batteries;Electrolyte;Interface engineering;Rare earth ions;Zinc anode

期刊：

Journal of Colloid and Interface Science

ISSN：

0021-9797

年：

2024

卷：

664

页码：

128-135

DOI：

10.1016/j.jcis.2024.03.034

基金类别：

CRediT authorship contribution statement Huaijun Zhang: Writing – original draft, Methodology, Investigation, Formal analysis, Data curation, Conceptualization. Hengyu Yang: Writing – original draft, Software, Data curation. Yongle Liang: Methodology, Formal analysis, Conceptualization. Fengjun Niu: Software, acquisition, Data curation. Guobao Xu: Writing – review & editing, Supervision. Xiaolin Wei: Writing – review & editing, Supervision. Liwen Yang: Writing – review & editing, Writing – original draft, Validation,

机构署名：

本校为其他机构

院系归属：

物理与电子工程学院

摘要：

Aqueous zinc-ion batteries (AZIBs) have become an ideal candidate for large-scale energy storage systems owing to their inherent safety and highly competitive capacity. However, severe dendrite growth and side reactions on the surface of zinc metal anodes lead to quick performance deterioration, seriously impeding the commercialization of AZIBs. In this work, a self-regulated zinc metal/electrolyte interface is constructed to solve these problems by incorporating the trivalent Gd(3+) additive with a lower effective reduction potential into the aqueous ZnSO(4) electrolyte. It is revealed that t...

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A self-regulated interface enabled by trivalent gadolinium ions toward highly reversible zinc metal anodes

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