Dual-functional surface hydroxyls and Brønsted acids in highly dispersed TiO2/Ti-HMS catalyst for efficient aerobic oxidation of cyclohexylamine to cyclohexanone oxime

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成果类型：

期刊论文

作者：

Shuilin Liu;Wenjin Ni*;Ning Liu;Xinde Tang;Suyun Wu;...

通讯作者：

Wenjin Ni

作者机构：

[Shuilin Liu; Ning Liu; Xinde Tang; Suyun Wu; Aiming Sun; Aiyang Li] School of chemical and environmental engineering, Hunan Institute of Technology, Hengyang 421002, China

College of Chemistry and Materials Science, Hengyang Normal University, Hengyang 421008, China

Key Laboratory of Functional Metal-Organic Compounds of Hunan Province, Hengyang 421008, China

[Wenjin Ni] College of Chemistry and Materials Science, Hengyang Normal University, Hengyang 421008, China<&wdkj&>Key Laboratory of Functional Metal-Organic Compounds of Hunan Province, Hengyang 421008, China

通讯机构：

[Wenjin Ni] C

College of Chemistry and Materials Science, Hengyang Normal University, Hengyang 421008, China<&wdkj&>Key Laboratory of Functional Metal-Organic Compounds of Hunan Province, Hengyang 421008, China

语种：

英文

期刊：

Journal of the Taiwan Institute of Chemical Engineers

ISSN：

1876-1070

年：

2026

卷：

180

页码：

106480

DOI：

10.1016/j.jtice.2025.106480

基金类别：

CRediT authorship contribution statement Shuilin Liu: Writing – original draft, Investigation, acquisition, Data curation. Wenjin Ni: Writing – review & editing, acquisition, Conceptualization. Ning Liu: acquisition, Formal analysis, Data curation. Xinde Tang: Supervision, Investigation. Suyun Wu: Software, Methodology, Investigation. Aiming Sun: Supervision, Formal analysis. Aiyang Li: Supervision, acquisition, Conceptualization.

机构署名：

本校为通讯机构

院系归属：

化学与材料科学学院

摘要：

Background The growing demand for ε-caprolactam, a key precursor for nylon-6 production, has driven strategic interest in developing cost-effective and environmentally benign approaches for cyclohexanone oxime synthesis. The growing demand for ε-caprolactam, a key precursor for nylon-6 production, has driven strategic interest in developing cost-effective and environmentally benign approaches for cyclohexanone oxime synthesis. Methods Ti-incorporated hexagonal mesoporous silica (TiO 2 /Ti-HMS) catalysts with tunable Ti/Si molar ratios were in...

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Dual-functional surface hydroxyls and Brønsted acids in highly dispersed TiO2/Ti-HMS catalyst for efficient aerobic oxidation of cyclohexylamine to cyclohexanone oxime

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