Fluorine-Decorated Metal-Organic Framework Separators Enable Ion-Screening Effects for Dendrite-Free Zinc Deposition

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成果类型：

期刊论文

作者：

Li, Zhongliang*;Hong, Zuchen;Yuan, Chenxu;Ouyang, Wenxi;Liu, Jinghua;...

通讯作者：

Li, Zhongliang;Lu, WH;Cai, YP

作者机构：

[Ouyang, Wenxi; Liu, Sai; Fang, Yiling; Liu, Jinghua; Wang, Wenbin; Lu, Weihong; Lei, Ke; Li, Ying; Yuan, Chenxu; Yang, Guiying; Hong, Zuchen; Li, Zhongliang; Tan, Liang] Hengyang Normal Univ, Sch Chem & Mat Sci, Hunan Engn Res Ctr Monitoring & Treatment Heavy Me, Hengyang 421008, Peoples R China.

[Li, Hui] Nanjing Univ Sci & Technol, Inst Computat Mol & Mat Sci, Sch Chem & Chem Engn, Nanjing 210094, Peoples R China.

[Zheng, Qifeng; Cai, Yuepeng] South China Normal Univ, Sch Chem, Guangzhou Key Lab Mat Energy Convers & Storage, Guangzhou 510006, Peoples R China.

通讯机构：

[Cai, YP ] S

[Lu, WH ; Li, ZL] H

Hengyang Normal Univ, Sch Chem & Mat Sci, Hunan Engn Res Ctr Monitoring & Treatment Heavy Me, Hengyang 421008, Peoples R China.

South China Normal Univ, Sch Chem, Guangzhou Key Lab Mat Energy Convers & Storage, Guangzhou 510006, Peoples R China.

语种：

英文

关键词：

aqueous zinc-ion batteries;dendrite-free;fluorine-decorated;homogenizing Zn2+ ion flux;metal-organic framework

期刊：

能源与环境材料(英文)

ISSN：

2575-0348

年：

2025

页码：

e70095

DOI：

10.1002/eem2.70095

基金类别：

Scientific Research Program of Hunan Education Department; Natural Science Foundation of Hunan Province [2024JJ6100]; Hengyang Normal University Science Foundation Project [2023QD22, 2024HSKFJJ019]; [23B0676]; [22B0723]

机构署名：

本校为第一且通讯机构

摘要：

Aqueous zinc-ion batteries (AZIBs) have emerged as a promising complement to lithium-ion batteries due to their inherent safety benefits. However, the cycle life of AZIBs is severely limited by the poor stability of zinc anodes, manifested in uncontrolled dendritic growth and persistent side reactions, which hinder wider application. Herein, we report an ion-selective separator (UIO-66-4F/GF) achieved by in situ growth of a fluorine-functionalized metal–organic framework (UIO-66-4F) onto commercial glass fiber (GF). The synergistic mechanism, ...

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Fluorine-Decorated Metal-Organic Framework Separators Enable Ion-Screening Effects for Dendrite-Free Zinc Deposition

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