Fe2O3/P-doped CoMoO4 electrocatalyst delivers efficient overall water splitting in alkaline media

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成果类型：

期刊论文

作者：

Wang, Bowen;Chen, Xiangxiong;He, Yingjian;Liu, Qin;Zhang, Xinxin;...

通讯作者：

Qian, Dong;Liu, JL;Waterhouse, GIN

作者机构：

[Liu, Qin; He, Yingjian; Liu, Jinlong; Qian, Dong; Chen, Xiangxiong; Wang, Bowen; Luo, Ziyu; Liu, JL; Zhang, Xinxin] Cent South Univ, Coll Chem & Chem Engn, Changsha 410083, Peoples R China.

[Chen, Xiangxiong] Yoening Tianci Min Changsha Technol Ctr, Changsha 410083, Peoples R China.

[V. Kennedy, John] GNS Sci, Natl Isotope Ctr, POB 30368, Lower Hutt 5010, New Zealand.

[Li, Junhua] Hengyang Normal Univ, Coll Chem & Mat Sci, Hengyang 421008, Peoples R China.

[Waterhouse, Geoffrey I. N.; Waterhouse, GIN] Univ Auckland, Sch Chem Sci, Auckland 1142, New Zealand.

通讯机构：

[Qian, D; Liu, JL ] C

[Waterhouse, GIN ] U

Cent South Univ, Coll Chem & Chem Engn, Changsha 410083, Peoples R China.

Univ Auckland, Sch Chem Sci, Auckland 1142, New Zealand.

语种：

英文

关键词：

Electrochemical reconstruction;CoMoO4-based catalyst;Phosphorization;Heterojunction;Overall water splitting

期刊：

Applied Catalysis B: Environmental

ISSN：

0926-3373

年：

2024

卷：

346

页码：

123741

DOI：

10.1016/j.apcatb.2024.123741

基金类别：

Acknowledgements This work was financially supported by National Natural Science Foundation of China (No. 51874359, 52103354, 21171174 and 21505035), the Natural Science Foundation of Hunan Province (2022JJ20084), the Science and Technology Innovation Program of Hunan Province (2023RC3034), and Research Faculty Startup of Central South University (202045020). GINW acknowledges funding support from the Royal Society Te Apārangi (via award of a James Cook Research Fellowship), the New Zealand Ministry of

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院系归属：

化学与材料科学学院

摘要：

Phosphorization of molybdates has been shown to promote hydrogen evolution reaction (HER) activity but is usually detrimental to oxygen evolution reaction (OER) activity, frustrating efforts to create bifunctional HER/OER electrocatalysts. Herein, we show that Fe2O3-modulated P-doped CoMoO4 on nickel foam (Fe-P-CMO) is an excellent bifunctional HER/OER electrocatalyst in alkaline media, with the adverse effect of phosphorization on the OER activity of CoMoO4 being countered via Fe2O3 introduction. An alkaline splitting electrolyser assembled di...

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Fe2O3/P-doped CoMoO4 electrocatalyst delivers efficient overall water splitting in alkaline media

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